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Recently I got a PS3 controller for Arkham City on PC and was pleasantly surprised that I could also use the controller to play games on my Galaxy Nexus! So far I tried it out with a SNES and GBA emulator and so far it's been working flawlessly!
Another great thing about it is that you can use the controller to operate your phone as well. For example, I can use it to navigate the phones menus and browse the web and place calls. It would be more interesting if my phone had a mini-HDMI output since I could use the controller as a remote while watching movies from my phone on the big screen.